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There are 16 nine-letter words beginning with OPTI

OPTICALLYoptically adv. Regarding or using optics.
OPTICAL adv. pertaining to sight.
OPTICIANSopticians n. Plural of optician.
OPTICIAN n. one who deals in optical goods.
OPTICISTSopticists n. Plural of opticist.
OPTICIST n. one engaged in the study of light and vision.
OPTIMALLYoptimally adv. In an optimal manner.
OPTIMAL adv. best, most desirable.
OPTIMATESoptimates n. Plural of optimate.
OPTIMATE n. a member of the aristocracy.
OPTIMISEDoptimised v. Simple past tense and past participle of optimise.
OPTIMISE v. to make as effective as possible, also OPTIMIZE.
OPTIMISERoptimiser n. Alternative spelling of optimizer.
OPTIMISER n. one who optimises, also OPTIMIZER.
OPTIMISESoptimises v. Third-person singular simple present indicative form of optimise.
OPTIMISE v. to make as effective as possible, also OPTIMIZE.
OPTIMISMSoptimisms n. Plural of optimism.
OPTIMISM n. a disposition that looks on the sunny side.
OPTIMISTSoptimists n. Plural of optimist.
Optimists n. Plural of Optimist.
OPTIMIST n. one who exhibits optimism.
OPTIMIZEDoptimized v. Simple past tense and past participle of optimize.
OPTIMIZE v. to make as effective as possible, also OPTIMISE.
OPTIMIZERoptimizer n. A person in a large business whose task is to maximize profits and make the business more efficient.
optimizer n. (Computing) A program that uses linear programming to optimize a process.
optimizer n. (Computing) A compiler or assembler that produces optimized code.
OPTIMIZESoptimizes v. Third-person singular simple present indicative form of optimize.
OPTIMIZE v. to make as effective as possible, also OPTIMISE.
OPTIONALSoptionals n. Plural of optional.
OPTIONAL n. an elective course of study.
OPTIONEESoptionees n. Plural of optionee.
OPTIONEE n. one who holds a legal option.
OPTIONINGoptioning v. Present participle of option.
OPTION v. to grant the act of choosing.

Scrabble words — in black are valid world wide — in RED are not valid in North America — in GREEN are valid only in North America.
Definitions are short excerpt from the WikWik.org and 1Word.ws.

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